Two-dimensional electronic photon-echo spectroscopy of photosynthetic complexes

• Antragsteller: Professor Dr. Wolfgang Domcke
• Fachliche Zuordnung: Theoretische Chemie: Elektronenstruktur, Dynamik, Simulation
• Förderung: Förderung von 2006 bis 2010
• Projektkennung: Deutsche Forschungsgemeinschaft (DFG) - Projektnummer 25637392

We have recently developed novel and particularly efficient algorithms for the calculation of femtosecond nonlinear spectra of complex systems. Here, we propose to numerically implement these methods for more demanding models of the excited-state dynamics of polyatomic molecules (e.g., conical intersections) as well as for the calculation of additional signals, e.g., multidimensional two- and three-pulse photon-echo spectroscopy and infrared emission. The project includes the development of a user-friendly code which allows the simulation of any third-order time- and frequency-resolved signal for a variety of models of the excited-state dynamics of polyatomic molecules.

• DFG-Verfahren: Sachbeihilfen